| |
|
|
Thursday, March 07, 20132:00 PM - 3:00 PMCNLS Conference Room (TA-3, Bldg 1690) Postdoc Seminar Effect of Localized Surface Plasmon Modes on Low-Dimensional Semiconductor-Metal Nanoparticle Hybrid Systems Charles CherquiUniversity of New Mexico / CNLS We examine the emergent physical properties of nanoscale (near-field) interactions between confined carriers/excitons and surface-plasmons in hybrid semiconductor-metal nanostructures. In particular this talk will discuss our theoretical study on both the charge carrier and exciton motion in one-dimensional semiconductor nanostructures (e.g., carbon nanotubes) in the presence of a single proximal metal nanoparticle. The effect of the charge-surface-plasmon interaction is treated in a method analogous to the polaron problem. This allows us to calculate zero-point dynamical quantum corrections to the charge-image potential which leads to the formation of a tunneling barrier controlling the charge transmission through the one-dimensional nanostructure. This effect could be exploited to create a nanoscale field effect transistor. Considering exciton transport, we show that the problem maps onto that of exciton scattering on an impurity state. We demonstrate that the surface-plasmon resonance leads to the formation of a localized band-gap state which dramatically influences the exciton-plasmon radiation pattern.
|